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Elucidating the intimate mechanism of NAD+ hydrogenation with phosphonic acid catalysed by Cp*Ir(pyridine-2-sulfonamidate) complexes

The reaction mechanism of nicotine amide dinucleotide hydrogenation (NAD+ to NADH) catalysed by Cp*Ir(pyridine-2-sulfonamidate) complexes in the presence of phosphonic acid has been elucidated. Multivariate kinetic experiments and NMR spectroscopy revealed that the enhanced performance of this class of catalysts arises from the hemilability of the pyridine ligand, which is displaced during P–H bond activation and facilitates the generation of the metal-hydride intermediate. Experimental resul...

How Photogenerated I2 Induces I‐rich Phase Formation in Lead Mixed Halide Perovskites

Bandgap tunability of lead mixed halide perovskites (LMHPs) is a crucial characteristic for versatile optoelectronic applications. Nevertheless, LMHPs show the formation of iodide-rich (I-rich) phase under illumination, which destabilizes the semiconductor bandgap and impedes their exploitation. Here, it is shown that how I2, photogenerated upon charge carrier trapping at iodine interstitials in LMHPs, can promote the formation of I-rich phase. I2 can react with bromide (Br−) in the perovskit...

Unified Approach for Damping Rate of Transient Laminar Flow: Experiments, Computational Fluid Dynamics, and One-Dimensional, and Global Models

Are Perovskite Solar Cells Reaching the Efficiency and Voltage Limits?

Hydrodynamics of laminar pipe flow through an extended partial blockage by CFD

In this paper, an advanced three-dimensional (3D) computational fluid dynamics (CFD) model is used to analyse the steady-state hydrodynamics of laminar flow through an extended partial blockage (PB) in a pressurised pipe. PB corresponds to one of the main faults affecting pipelines. In fact, it reduces its carrying capacity with economic consequences, and as it does not give rise to any external evidence, its detection can be very challenging. The performance of the model is evaluated by comp...

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